I think a lot of people on this thread are over-thinking the over-improvement. There's an old engineering term that's tried and true, "Keep it simple stupid." If it's truly an over-improvement due primarily to size (which I think is where you're going with this), then the market will only give you a marginal premium for that additional square footage. So what does that GLA adjustment look like?
Well, first, you must (and I can't emphasize this enough) find a bracketing comparable or two. It will most likely come from a superior neighborhood. And that neighborhood will command a higher land value. Estimate it. It's your location adjustment. Next, select the largest and most similar home sales in your neighborhood. Apply the location adjustment to all of them. Account for all other factors like bath count, pool, outdoor living, parking, etc. You should probably go ahead and deduct any concessions. What you're left with is the GLA adjustment. This is where you play with the numbers. Pair your bracketing comparable with all of the other comparables to determine the GLA adjustment/sf that best smooths the data. And what you'll find is a relatively low GLA adjustment which effectively illustrates the marginal premium the market is willing to pay for that additional square footage. It works every time.
Hopefully, your conclusion of market value will be close to the top of your neighborhood, maybe even a little higher (and just because it's higher doesn't make it wrong). Explain the steps you took in detail to your client in the narrative. If you want to get fancy, cite the relationship between the largest property sale from another neighborhood to the predominant and see if that relationship is similar to your conclusion. That would add some credibility. Over-improvements are always subjective because the market reacts differently on any given day. But these are the steps you can take to try and apply some logic to it. All y'all can disagree but this is how I've handled it.
Remember, residential buyers are unsophisticated and they're not logical like commercial investors. But they will know not to pay as much for your home as they would for a similar home in a superior neighborhood. That's the relationship you are trying to quantify.